期刊
NANOPHOTONICS
卷 10, 期 8, 页码 1943-1965出版社
WALTER DE GRUYTER GMBH
DOI: 10.1515/nanoph-2020-0681
关键词
coherent dynamics; exciton dynamics; perovskite nanocrystals; spin dynamics; ultrafast spectroscopy
资金
- National Key R&D Program of China [2017YFA0303700, 2018YFA0209101]
- National Science Foundation of China [21922302, 21873047, 11904168, 91833305, 91850105]
- Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD)
- Fundamental Research Funds for the Central University
Perovskite semiconductor nanocrystals have shown promise in optoelectronic applications, with recent research focusing on their photoinduced carrier dynamics. The dynamics of carrier generation, recombination, and transport play essential roles in the performance of devices such as light-emitting diodes and solar cells. Spin dynamics and coherent exciton dynamics are important for potential applications in quantum information technology, though there are still controversial results and unresolved origins to be addressed.
Perovskite semiconductor nanocrystals have emerged as a promising family of materials for optoelectronic applications including light-emitting diodes, lasers, light-to-electricity convertors and quantum light emitters. The performances of these devices are fundamentally dependent on different aspects of the excited-state dynamics in nanocrystals. Herein, we summarize the recent progress on the photoinduced carrier dynamics studied by a variety of time-resolved spectroscopic methods in perovskite nanocrystals. We review the dynamics of carrier generation, recombination and transport under different excitation densities and photon energies to show the pathways that underpin the photophysics for light-emitting diodes and solar cells. Then, we highlight the up-to-date spin dynamics and coherent exciton dynamics being manifested with the exciton fine levels in perovskite semiconductor nanocrystals which are essential for potential applications in quantum information technology. We also discuss the controversial results and the possible origins yet to be resolved. In-depth study toward a comprehensive picture of the excited-state dynamics in perovskite nanocrystals may provide the key knowledge of the device operation mechanism, enlighten the direction for device optimization and stimulate the adventure of new conceptual devices.
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