Rise and fall of Landau's quasiparticles while approaching the Mott transition

Landau suggested that the low-temperature properties of metals can be understood in terms of long-lived quasiparticles with all complex interactions included in Fermi-liquid parameters, such as the effective mass m(star). Despite its wide applicability, electronic transport in bad or strange metals and unconventional superconductors is controversially discussed towards a possible collapse of the quasiparticle concept. Here we explore the electrodynamic response of correlated metals at half filling for varying correlation strength upon approaching a Mott insulator. We reveal persistent Fermi-liquid behavior with pronounced quadratic dependences of the optical scattering rate on temperature and frequency, along with a puzzling elastic contribution to relaxation. The strong increase of the resistivity beyond the Ioffe-Regel-Mott limit is accompanied by a 'displaced Drude peak' in the optical conductivity. Our results, supported by a theoretical model for the optical response, demonstrate the emergence of a bad metal from resilient quasiparticles that are subject to dynamical localization and dissolve near the Mott transition.

Automated summary

This study reveals the persistent Fermi-liquid behavior in correlated metals at half filling for varying correlation strength upon approaching a Mott insulator, showing pronounced quadratic dependences and a puzzling elastic contribution. The emergence of a bad metal from resilient quasiparticles near the Mott transition is demonstrated, supported by a theoretical model for the optical response.