期刊
JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS
卷 521, 期 -, 页码 -出版社
ELSEVIER
DOI: 10.1016/j.jmmm.2020.167505
关键词
Two-dimensional quantum antiferromagnet; Spin-1/2 Heisenberg square-lattice model; Rotation-invariant Green's function method
资金
- Russian Foundation for Basic Research [19-02-00509]
- Russian Science Foundation [18-12-00133]
In this study, we investigate the spin excitations in an ordered square quantum antiferromagnet under a magnetic field, predicting the emergence of three modes and a hybridization effect due to the field. The theoretical predictions are compared with exact diagonalization and neutron scattering experiments to confirm the validity of the model.
We predict that spin-waves in an ordered square quantum antiferromagnet in a magnetic field (h) perpendicular to antiferromagnetic plane may demonstrate three modes of spin excitations. Starting from the self-consistent rotation-invariant Green's function method, a new mean-field theory is constructed for h not equal 0. The method preserves the translational and the axial symmetries, and provides exact fulfillment of the single-site constraint for each of the three modes. We examine the dynamical structure factors S-alpha alpha(k, omega),alpha(beta) = x, y, z. It is shown, that the introduction of h leads to the hybridization of two degenerate spin modes due to the appearance of a non-diagonal on alpha, beta spin-spin Green's functions. The comparison of the theory with the exact diagonalization study and with results on inelastic neutron scattering experiments is discussed at T = 0. We discuss also the correspondence of the present theory to the existing theories, which allow only two spin excitations modes for the total S(k, omega).
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