期刊
JOURNAL OF ENVIRONMENTAL SCIENCES
卷 100, 期 -, 页码 1-10出版社
SCIENCE PRESS
DOI: 10.1016/j.jes.2020.06.004
关键词
PM2.5; Seasonal variations; Chemical composition; Source apportionment; Pollution evolution
资金
- National Natural Science Foundation of China [41805095, 41705113, 14877312]
- Sichuan Science and Technology Program [7018SZ0788, 2019YFS0476]
- National Research Program for Key Issues in Air Pollution Control [DQGG0101]
- Beijing Major Science and Technology Project [Z181100005418014]
Following the implementation of strict clean air policies in Beijing, the study found a decrease in PM2.5 concentration, with spring having the highest levels. Secondary nitrate and vehicular emissions were identified as the main sources of PM2.5. Contributions from coal combustion decreased significantly, while contributions from EC and NO3- increased during weekends.
Following the implementation of the strictest clean air policies to date in Beijing, the physicochemical characteristics and sources of PM2.5 have changed over the past few years. To improve pollution reduction policies and subsequent air quality further, it is necessary to explore the changes in PM2.5 over time. In this study, over one year (2017-2018) field study based on filter sampling (TH-150C; Wuhan Tianhong, China) was conducted in Fengtai District, Beijing, revealed that the annual average PM2.5 concentration (64.8 +/- 43.1 mu g/m(3)) was significantly lower than in previous years and the highest PM2.5 concentration occurred in spring (84.4 +/- 59.9 mu g/m(3)). Secondary nitrate was the largest source and accounted for 25.7% of the measured PM2.5. Vehicular emission, the second largest source (17.6%), deserves more attention when considering the increase in the number of motor vehicles and its contribution to gaseous pollutants. In addition, the contribution from coal combustion to PM2.5 decreased significantly. During weekends, the contribution from EC and NO3- increased whereas the contributions from SO42-, OM, and trace elements decreased, compared with weekdays. During the period of residential heating, PM2.5 mass decreased by 23.1%, compared with non -heating period, while the contributions from coal combustion and vehicular emission, and related species increased. With the aggravation of pollution, the contribution of vehicular emission and secondary sulfate increased and then decreased, while the contribution of NO3- and secondary nitrate continued to increase, and accounted for 34.0% and 57.5% of the PM2.5 during the heavily polluted days, respectively. (C) 2020 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V.
作者
我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。
推荐
暂无数据