期刊
CHEMICAL RECORD
卷 21, 期 4, 页码 841-857出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/tcr.202000186
关键词
Photoelectrocatalysis; oxidation; organic synthesis; catalytic performance; mechanism
资金
- National Natural Science Foundation of China [21771021, 21822501, 21978021, 22061130206]
- Beijing Municipal Natural Science Foundation [JQ20003]
- Newton Advanced Fellowship award [NAF\R1\201285]
- Fok Ying-Tong Education Foundation [171008]
- Beijing Nova Program [xx2018115]
- Measurements Fund of Beijing Normal University
- Fundamental Research Funds for the Central Universities
The rapid development of radical chemistry has led to the emergence of innovative strategies for organic synthesis, among which photoelectrocatalysis (PEC) has received considerable attention as a promising approach. Although many catalytic reactions face challenges such as high overpotential and poor conversion efficiency, scientists are actively seeking solutions to enhance the accessibility and further development of photoelectrocatalytic technology for specific chemical bond formation and catalytic system fabrication.
The rapid development of radical chemistry has spurred several innovative strategies for organic synthesis. The novel approaches for organic synthesis play a critical role in promoting and regulating the single-electron redox activity. Among them, photoelectrocatalysis (PEC) has attained considerable attention as the most promising strategy to convert organic compounds into fine chemicals. This review highlights the current progress in organic synthesis through PEC, including various catalytic reactions, catalyst systems and practical applications. The numerous catalytic reactions suffer the high overpotential and poor conversion efficiency, depending on the design of electrolyzers and the reaction mechanisms. We also considered the recent developments with special emphasis on scientific problems and efficient solutions, which enhance accessibility to utilize and further develop the photoelectrocatalytic technology for the specific chemical bonds formation and the fabrication of numerous catalytic systems.
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