期刊
CATALYSIS COMMUNICATIONS
卷 151, 期 -, 页码 -出版社
ELSEVIER
DOI: 10.1016/j.catcom.2021.106279
关键词
Layered double hydroxide; Hydroxymethylfurfural; Diformylfuran; Catalytic oxidation; Nickel; Manganese
资金
- Jiangsu Key Laboratory of Advanced Catalytic Materials and Technology [BM2012110]
- Research Foundation of Jiangsu Educational Committee [20KJA530003]
- Jiangsu Key Laboratory of Biomass Energy and Material [JSBEM202018]
- Key Technology R&D Program of Changzhou [CE20205054]
- Qinglan Project of Jiangsu Province
- Natural Science Foundation of Jiangsu Province of China [BK20181461]
Ni3Mn-LDH has been found to be an efficient catalyst for the oxidation of HMF to DFF using molecular oxygen. Both Ni2+ and Mn3+ species in the structure were suggested as active sites for the oxidation of HMF, showing a synergistic effect in the transformation process. The catalyst exhibited impressive catalytic performance, good stability, and recyclability.
NiMn layered double hydroxide (Ni3Mn-LDH) has been found to be an efficient catalyst for the oxidation of 5-hydroxymethylfurfural (HMF) to 2,5-diformylfuran (DFF) using molecular oxygen as the sole oxidant. Various reaction conditions on the oxidation have been investigated, and impressive catalytic performance, good stability and recyclability have been observed for Ni3Mn-LDH. Both of Ni2+ and Mn3+ species in the structure were proposed to be the catalytically active site for the aerobic oxidation of HMF, and the two species in the transformation exhibited synergistic effect.
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