Metal Halide Perovskites for Laser Applications

Metal halide perovskites have drawn tremendous attention in optoelectronic applications owing to the rapid development in photovoltaic and light-emitting diode devices. More recently, these materials are demonstrated as excellent gain media for laser applications due to their large absorption coefficient, low defect density, high charge carrier mobility, long carrier diffusion length, high photoluminescence quantum yield, and low Auger recombination rate. Despite the great progress in laser applications, the development of perovskite lasers is still in its infancy and the realization of electrically pumped lasers has not yet been demonstrated. To accelerate the development of perovskite-based lasers, it is important to understand the fundamental photophysical characteristics of perovskite gain materials. Here, the structure and gain behavior in various perovskite materials are discussed. Then, the effects of charge carrier dynamics and electron-phonon interaction on population inversion in different types of perovskite materials are analyzed. Further, recent advances in perovskite-based lasers are also highlighted. Finally, a perspective on perovskite material design is presented and the remaining challenges of perovskite lasers are discussed.

Automated summary

Metal halide perovskites are gaining attention in optoelectronic applications due to their properties such as large absorption coefficient, low defect density, and high charge carrier mobility. While progress has been made in perovskite-based lasers, the development is still in its early stages and electrically pumped lasers have not been realized yet. Understanding the fundamental photophysical characteristics of perovskite gain materials is crucial to accelerating their development in laser applications.