4.8 Article

Antiferromagnetic switching driven by the collective dynamics of a coexisting spin glass

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SCIENCE ADVANCES
卷 7, 期 2, 页码 -

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AMER ASSOC ADVANCEMENT SCIENCE
DOI: 10.1126/sciadv.abd8452

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  1. Center for Novel Pathways to Quantum Coherence in Materials, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences
  2. Gordon and Betty Moore Foundation's EPiQS Initiative [GBMF9067]
  3. Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]
  4. National Science Foundation [DMR-1644779]
  5. State of Florida
  6. NSF [DMR-1742928]

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It is demonstrated that the coexistence of spin glass and antiferromagnetic order allows a novel mechanism for switching the antiferromagnet Fe1/3 + delta NbS2, rooted in the electrically stimulated collective winding of the spin glass. This manipulation of antiferromagnetic spin textures using the collective dynamics of a spin glass opens up new material platforms for antiferromagnetic spintronics with complex magnetic textures.
The theory behind the electrical switching of antiferromagnets is premised on the existence of a well-defined broken symmetry state that can be rotated to encode information. A spin glass is, in many ways, the antithesis of this state, characterized by an ergodic landscape of nearly degenerate magnetic configurations, choosing to freeze into a distribution of these in a manner that is seemingly bereft of information. Here, we show that the coexistence of spin glass and antiferromagnetic order allows a novel mechanism to facilitate the switching of the antiferromagnet Fe1/3 + delta NbS2, rooted in the electrically stimulated collective winding of the spin glass. The local texture of the spin glass opens an anisotropic channel of interaction that can be used to rotate the equilibrium orientation of the antiferromagnetic state. Manipulating antiferromagnetic spin textures using a spin glass' collective dynamics opens the field of antiferromagnetic spintronics to new material platforms with complex magnetic textures.

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