4.6 Article

Lattice Resonances Induced by Periodic Vacancies in Arrays of Nanoparticles

期刊

ACS PHOTONICS
卷 8, 期 1, 页码 360-368

出版社

AMER CHEMICAL SOC
DOI: 10.1021/acsphotonics.0c01672

关键词

lattice resonances; vacancy; periodic arrays; nanoparticle arrays; plasmons; plasmonic crystals

资金

  1. U.S. National Science Foundation [ECCS-1710697]
  2. U.S. National Science Foundation
  3. New Mexico Space Grant Consortium
  4. Department of Energy Computational Science Graduate Fellowship [DE-SC0020347]
  5. U.S. Department of Energy (DOE) [DE-SC0020347] Funding Source: U.S. Department of Energy (DOE)

向作者/读者索取更多资源

Periodic arrays of nanoparticles can support lattice resonances, with the potential to induce vacancies in the array resulting in unique lattice resonances. Through a comprehensive analysis using a coupled dipole approach, it was found that these vacancy-induced lattice resonances have subradiant character and originate from symmetry breaking caused by the vacancies. The study also explores the possibility of implementing arrays with vacancies made of nanocylinders in a homogeneous dielectric environment to control the optical response of nanostructures.
Periodic arrays of nanoparticles are capable of supporting lattice resonances, collective modes arising from the coherent interaction of the particles in the array. These resonances, whose spectral position is determined by the array periodicity, are spectrally narrow and lead to strong optical responses, making them useful for a wide range of applications, from nanoscale light sources to ultrasensitive biosensors. Here, we report that, by removing particles from an array in a periodic fashion, it is possible to induce lattice resonances at wavelengths commensurate with the periodicity of these vacancies, which would otherwise not be present in the system. Using a coupled dipole approach, we perform a comprehensive analysis of how the properties of these vacancy-induced lattice resonances depend on the array periodicity, the particle size, and the number of vacancies per unit of area. Furthermore, we find that these lattice resonances have a subradiant character and originate from the symmetry breaking introduced in the unit cell by the presence of the vacancies. Finally, we investigate a potential implementation of an array with vacancies made of nanocylinders embedded in a homogeneous dielectric environment. The results of this work serve to advance our understanding of lattice resonances and provide an alternative method for controlling the optical response of periodic arrays of nanostructures.

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