4.8 Article

New particle formation in the remote marine boundary layer

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NATURE COMMUNICATIONS
卷 12, 期 1, 页码 -

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NATURE RESEARCH
DOI: 10.1038/s41467-020-20773-1

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资金

  1. Office of Biological and Environmental Research
  2. Atmospheric System Research (ASR) program (Office of Biological and Environmental Research of US DOE) [DE-SC0020259, DE-AC0298CH10886]
  3. NASA NAAMES project within the Earth Venture Suborbital-2 Program [NNH13ZDA001N-EVS2]
  4. U.S. Department of Energy (DOE) [DE-SC0020259] Funding Source: U.S. Department of Energy (DOE)

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Marine low clouds play a crucial role in the climate system, with their properties being sensitive to cloud condensation nuclei concentrations. New particle formation is a major source of cloud condensation nuclei globally, and evidence shows that it regularly occurs in the upper part of the remote marine boundary layer following cold front passages, impacting marine low clouds.
Marine low clouds play an important role in the climate system, and their properties are sensitive to cloud condensation nuclei concentrations. While new particle formation represents a major source of cloud condensation nuclei globally, the prevailing view is that new particle formation rarely occurs in remote marine boundary layer over open oceans. Here we present evidence of the regular and frequent occurrence of new particle formation in the upper part of remote marine boundary layer following cold front passages. The new particle formation is facilitated by a combination of efficient removal of existing particles by precipitation, cold air temperatures, vertical transport of reactive gases from the ocean surface, and high actinic fluxes in a broken cloud field. The newly formed particles subsequently grow and contribute substantially to cloud condensation nuclei in the remote marine boundary layer and thereby impact marine low clouds. Globally, new particle formation represents a major source of cloud condensation nuclei. Here, the authors present evidence of frequent occurrence of new particle formation in the upper part of remote marine boundary layer following cold front passages.

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