Burst-mode dual-comb spectroscopy

We introduce a new, to the best of our knowledge, modality of dual-comb spectroscopy (DCS) that enables a simplified and powerful new approach for time-resolved measurements with increased acquisition rates. This burst mode form of DCS relies on the multiplexing of each probe pulse into a short train of pulses. With this approach we demonstrate a time-resolved series of absorption-based spectroscopic measurements of a laser-induced plasma using only a single laser ablation shot and identify 22 Nd lines not previously reported in the literature. The transmission spectra spanned 3.1 THz and were acquired at an effective acquisition rate of 25 kHz with 40 mu s time resolution. This simple modification to similar to 100 MHz level dual-comb systems provides a flexible approach for studying transient and low-duty-cycle events such as laser-induced plasmas, combustion, and explosive reactions. (C) 2021 Optical Society of America

Automated summary

The study presents a new modality of dual-comb spectroscopy that offers a simplified and powerful approach for time-resolved measurements with increased acquisition rates. By multiplexing each probe pulse into a short train of pulses, a time-resolved series of absorption-based spectroscopic measurements was demonstrated, identifying 22 Nd lines not previously reported. This modification to dual-comb systems enables flexible studying of transient and low-duty-cycle events.