4.8 Article

A charge-density-wave topological semimetal

期刊

NATURE PHYSICS
卷 17, 期 3, 页码 381-+

出版社

NATURE PORTFOLIO
DOI: 10.1038/s41567-020-01104-z

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资金

  1. DOE [DE-SC0016239]
  2. NSF EAGER [DMR 1643312]
  3. NSF-MRSEC [DMR-2011750, DMR-142051]
  4. Simons Investigator grant [404513]
  5. ONR [N00014-14-1-0330, N00014-20-1-2303]
  6. BSF Israel US Foundation [2018226]
  7. Packard Foundation
  8. Schmidt Fund for Innovative Research
  9. John Simon Guggenheim Memorial Foundation
  10. National Natural Science Foundation of China [11974395, U1932217, 11974246]
  11. Chinese Academy of Sciences (CAS) [XDB33000000]
  12. Center for Materials Genome
  13. CAS Pioneer Hundred Talents Program
  14. DFG through the priority program SPP1666 (Topological Insulators)
  15. ERC [291472, 742068-TOPMAT]
  16. Deutsche Forschungsgemeinschaft DFG [SFB 1143]
  17. Shanghai high-repetition-rate XFEL and extreme light facility (SHINE)

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The study demonstrates that (TaSe4)(2)I is a Weyl semimetal with 24 pairs of Weyl nodes at room temperature, and also exhibits an established charge-density wave instability. The charge-density wave in (TaSe4)(2)I couples the bulk Weyl points and opens a bandgap, providing a pathway for exploring the interplay of correlations and topology in a solid-state material.
Topological physics and strong electron-electron correlations in quantum materials are typically studied independently. However, there have been rapid recent developments in quantum materials in which topological phase transitions emerge when the single-particle band structure is modified by strong interactions. Here we demonstrate that the room-temperature phase of (TaSe4)(2)I is a Weyl semimetal with 24 pairs of Weyl nodes. Owing to its quasi-one-dimensional structure, (TaSe4)(2)I also hosts an established charge-density wave instability just below room temperature. We show that the charge-density wave in (TaSe4)(2)I couples the bulk Weyl points and opens a bandgap. The correlation-driven topological phase transition in (TaSe4)(2)I provides a route towards observing condensed-matter realizations of axion electrodynamics in the gapped regime, topological chiral response effects in the semimetallic phase, and represents an avenue for exploring the interplay of correlations and topology in a solid-state material.

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