期刊
NATURE MATERIALS
卷 20, 期 4, 页码 463-+出版社
NATURE PORTFOLIO
DOI: 10.1038/s41563-020-00884-2
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资金
- JST PRESTO 'Scientific Innovation for Energy Harvesting Technology' [JPMJPR17R5]
- JST CREST 'Creation of Innovative Core Technologies for Nano-enabled Thermal Management' [JPMJCR17I1]
- New Energy and Industrial Technology Development Orgnization (NEDO) 'Mitou' challenge 2050 [P14004]
- Japan Society for the Promotion of Science (JSPS) [JP18J02115]
This study utilizes the Seebeck effect to drive transverse thermoelectric generation, which shows great potential for energy harvesting and heat sensing applications, especially with the orthogonal geometry in the heat-to-charge current conversion. By hybridizing Seebeck effect and anomalous Hall effect in a closed circuit comprising thermoelectric and magnetic materials, a similar symmetry to the anomalous Nernst effect can be achieved in transverse thermoelectric generation. The Seebeck-effect-driven transverse thermopower is found to be several orders of magnitude larger than the anomalous-Nernst-effect-driven thermopower, indicating a promising unconventional approach for developing applications of transverse thermoelectric generation.
When a temperature gradient is applied to a closed circuit comprising two different conductors, a charge current is generated via the Seebeck effect(1). Here, we utilize the Seebeck-effect-induced charge current to drive 'transverse' thermoelectric generation, which has great potential for energy harvesting and heat sensing applications owing to the orthogonal geometry of the heat-to-charge-current conversion(2-9). We found that, in a closed circuit comprising thermoelectric and magnetic materials, artificial hybridization of the Seebeck effect into the anomalous Hall effect(10) enables transverse thermoelectric generation with a similar symmetry to the anomalous Nernst effect(11-27). Surprisingly, the Seebeck-effect-driven transverse thermopower can be several orders of magnitude larger than the anomalous-Nernst-effect-driven thermopower, which is clearly demonstrated by our experiments using Co2MnGa/Si hybrid materials. The unconventional approach could be a breakthrough in developing applications of transverse thermoelectric generation.
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