期刊
JOURNAL OF PHYSICS-CONDENSED MATTER
卷 33, 期 7, 页码 -出版社
IOP PUBLISHING LTD
DOI: 10.1088/1361-648X/abc729
关键词
heavy fermion; metamagnetism; Lifshitz transition; strongly correlated electrons
资金
- NSERC [RGPIN-2019-06446]
- HFML-RU/NWO, member of the European Magnetic Field Laboratory (EMFL)
Through a combination of experimental measurements and theoretical calculations, a correlation between the metamagnetic transition and Fermi surface structure in UPt3 material has been discovered, which may affect its superconducting properties. The magnetization arises from the non-linear spin-splitting of Fermi bands, explaining the non-linear field dependence of quantum oscillation frequencies.
Comparing quantum oscillation measurements, dc magnetoresistance measurements, and Fermi surfaces obtained from LDA calculations, we argue that the metamagnetic transition of UPt3, which occurs at an applied field mu H-circle(M) similar to 20 T, coincides with a Lifshitz transition at which an open orbit on the band 2 hole-like Fermi surface becomes closed for one spin direction. At low field, proximity of the Fermi energy to this particular van Hove singularity may have implications for the superconducting pairing potential of UPt3. In our picture the magnetization comes from non-linear spin-splitting of the heavy fermion bands. In support of this, we show that the non-linear field dependence of a particular quantum oscillation frequency can be fitted by assuming that the corresponding extremal Fermi surface area is proportional to the magnetization. In addition, below H-M, we find in our LDA calculations a new, non-central orbit on band 1, whose non-linear behaviour explains a field-dependent frequency recently observed in magnetoacoustic quantum oscillation measurements.
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