期刊
ENVIRONMENTAL POLLUTION
卷 268, 期 -, 页码 -出版社
ELSEVIER SCI LTD
DOI: 10.1016/j.envpol.2020.115848
关键词
Antarctica; Dome A; Heavy metals; Anthropogenic pollution
资金
- Chinese Arctic and Antarctic Administration [CXPT2020012]
- 333 Project of Jiangsu Province [BRA2020030]
- National Natural Science Foundation of China [41830644, 91837102, 41771031, 41622605]
The study found that the concentrations of heavy metals in Dome A in Antarctica were influenced by human activities, mainly from Australia and South America. By analyzing the relationship between trace element fluxes and sea ice concentration, sea surface temperature, and air temperature, it was revealed that the deposition and transport of atmospheric aerosols at Dome A were influenced by circum-Antarctic atmospheric circulations.
Antarctic trace element records could provide important insights into the impact of human activities on the environment over the past few centuries. In this study, we investigated the atmospheric concentrations of 14 representative heavy metals (Al, As, Cd, Co, Cu, Fe, K, Mg, Mn, Pb, Sb, Sr, Tl and V) from 174 samples collected in a 4-m snow pit at Dome Argus (Dome A) on the East Antarctic Plateau, covering the period from 1950 to 2016 A.D. We found great variability in the annual concentration of all metals. The crustal enrichment factors suggest that the concentrations of some heavy metals (Cd, Sb, Cu, As and Pb) were likely influenced by anthropogenic activities in recent decades. An analysis of source regions suggests that heavy metal pollution at Dome A was largely caused by human activities in Australia and South America (e.g. mining production, leaded gasoline). Based on the relationship between the trace elements fluxes and sea ice concentration (SIC), sea surface temperature (SST) and annual mean air temperature at 2 m above the ground (T-2m), our analysis shows that deposition and transport of atmospheric aerosol at Dome A were influenced by circum-Antarctic atmospheric circulations. (C) 2020 Elsevier Ltd. All rights reserved.
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