期刊
ATMOSPHERIC RESEARCH
卷 248, 期 -, 页码 -出版社
ELSEVIER SCIENCE INC
DOI: 10.1016/j.atmosres.2020.105247
关键词
Biomass burning; Carbonaceous matter; Brown carbon; Fugitive emission
资金
- second Tibetan Plateau Scientific Expedition and Research Program [2019QZKK0605]
- China National Nature Science Foundation [41922057, 41830641]
- Chinese Academy of Science [XDA23010100]
Biomass burning is a major source of ambient and indoor PM2.5, with carbonaceous matters being of significant concern for health and climate impacts. Fugitive emissions from biomass burning can lead to severe indoor air pollution.
Biomass burning constitutes a major source of ambient PM2.5 but also a predominant source of indoor PM2.5. Carbonaceous matters, such as organic carbon (OC), elemental carbon (EC), black carbon, and brown carbon (BrC), are major components of PM2.5, and are of broad concern due to their significant impacts on health and climate patterns. In this study, we took simultaneous indoor and outdoor emission measurements to quantify pollutant emission factors (EFs) of carbonaceous matters, including the stack and fugitive EFs, from the real world biomass burning in rural households. Modified combustion efficiency, fuel moisture, burning rates, and chimney gas velocity explained 45-71% of variations in the field-based emission factors. BrC (measured at 370 nm, and estimated based on the specific attenuation coefficients-16.6 m(2)/g at 880 nm and 39.5 m(2)/g at 370 nm) comprised up to similar to 20% of all OC. Fractions of fugitive emissions of the total reached as high as 44-48%. Fugitive emissions would result in very high peak concentrations of approximately tens of mg/m(3), leading to severe indoor air pollution. The study clearly demonstrates that the simultaneous studies on indoor and outdoor emissions and air quality is crucial to understand mechanisms of the environmental impacts of internal combustion sources.
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