期刊
DALTON TRANSACTIONS
卷 45, 期 30, 页码 12114-12118出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6dt01737a
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资金
- Kurata Memorial Hitachi Science and Technology Foundation
- Core Research for Evolutionary Science and Technology of Japan Science and Technology Agency
- Japan Society for the Promotion of Science (JSPS) [15H05424]
- Japan Society for the Promotion of Science through Program for Leading Graduate Schools (MERIT)
- Grants-in-Aid for Scientific Research [15H05424] Funding Source: KAKEN
A new phase of oxyhydride NdNiOxHy with a defect-fluorite structure was obtained by a soft chemical reaction of NdNiO3 epitaxial thin films on a substrate of SrTiO3 (100) with CaH2. The epitaxial relationship of this phase relative to SrTiO3 could be controlled by changing the reaction temperature. At 240 degrees C, NdNiOxHy grew with a [001] orientation, forming a thin layer of infinite-layer NdNiO2 at the interface between the NdNiOxHy and the substrate. Meanwhile, a high-temperature reaction at 400 degrees C formed [110]-oriented NdNiOxHy without NdNiO2.
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