期刊
NATURE CATALYSIS
卷 3, 期 10, 页码 775-786出版社
NATURE RESEARCH
DOI: 10.1038/s41929-020-00512-x
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资金
- Christian Doppler Research Association
- Austrian Federal Ministry for Digital and Economic Affairs
- National Foundation for Research, Technology and Development
- OMV Group
Substantial progress has recently been made in the general understanding of the interfacial CO(2)reduction reaction (CO2RR) in electro- and photocatalysis, but the influence of the local chemical environment and its effects on the catalytic interface at the molecular level remains largely elusive. Here, we introduce a classification scheme to group different aspects influencing the interfacial CO2RR thermodynamics and kinetics. This categorization allows a systematic survey of the literature focusing on the local chemical environment encompassing surface effects (adsorbates, support), solution interactions (electrolyte constituents) and three-dimensional chemical surroundings (polymers, metal organic frameworks (MOFs), covalent organic frameworks (COFs)). The review concludes with an outlook discussing possible future concepts for next-generation electrocatalytic and photocatalytic CO2RR.
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