4.8 Article

MXene Ti3C2 memristor for neuromorphic behavior and decimal arithmetic operation applications

期刊

NANO ENERGY
卷 79, 期 -, 页码 -

出版社

ELSEVIER
DOI: 10.1016/j.nanoen.2020.105453

关键词

MXene Ti3C2; Ag nanoparticle; Memristor; EPSC; Decimal arithmetic

资金

  1. National Natural Science Foundation of China [61674050, 61874158]
  2. Outstanding Youth Project of Hebei Province [F2016201220]
  3. Outstanding Youth Cultivation Project of Hebei University [2015JQY01]
  4. Project of Science and Technology Activities for Overseas Researcher [CL 201602]
  5. Project of Distinguished Young of Hebei Province [A2018201231]
  6. Support Program for the Top Young Talents of Hebei Province [70280011807]
  7. Training and Introduction of High-Level Innovative Talents of Hebei University [801260201300]
  8. Hundred Persons Plan of Hebei Province [E2018050004, E2018050003]
  9. Supporting Plan for 100 Excellent Innovative Talents in Colleges and Universities of Hebei Province [SLRC2019018]
  10. opening project of Key Laboratory of Microelectronic Devices & Integrated Technology, Institute of Microelectronics, Chinese Academy of Sciences

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This study presents a facile method to improve the electronic performance of MXene Ti3C2 memristor by Ag nanoparticle doping. The doping method exhibits bidirectional continuous current transition behavior and has the potential to implement decimal arithmetic operations.
MXene Ti3C2, as the emerging member of two-dimensional (2D) materials family, has been applied to memristor and exhibited fast pulse modulation time and miniaturization size. However, the current abrupt behavior of switching processes hampered its further applications as a neuro-bionic device. Here, we present a facile method to improve the electronic performance of 2D MXene Ti3C2-based memristor by Ag nanoparticle doping. Compared to the pure Ti3C2 device, the Ag nanoparticle doping method exhibits a bidirectional continuous current transition behavior. Then, the variation trend of excitatory postsynaptic current (EPSC) was analysis in detail, and the transition rule of short-term potentiation (STP) to long-term potentiation (LTP) was systematically summarized. More interestingly, the energy consumption of generate one spike in unit device is as low as 0.35pj. And the memristor has ability to implement decimal arithmetic operations such as addition and multiplication. Exploration of the microstructure and finite element analysis (FEA) shows that the atomic vacancies capture the metal ions to form the filaments. This work provides a facile method to improve the electronic neuromorphic performance of MXene Ti3C2 memristor, which will considerably promote the diversification development of 2D materials in the field of neuro-morphology chips and greatly enhance the practicability of 2D materials.

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