4.7 Article

Uncovering Non-Fermi-Liquid Behavior in Hund Metals: Conformal Field Theory Analysis of an SU(2) x SU(3) Spin-Orbital Kondo Model

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PHYSICAL REVIEW X
卷 10, 期 3, 页码 -

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AMER PHYSICAL SOC
DOI: 10.1103/PhysRevX.10.031052

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资金

  1. Deutsche Forschungsgemeinschaft under Germany's Excellence Strategy [EXC-2111-390814868, LE3883/2-1]
  2. U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0012704]
  3. National Science Foundation [DMR-1733071]
  4. U.S. Department of Energy, Office of Science, Basic Energy Sciences, Computational Materials Science Program through the Center for Computational Design of Functional Strongly Correlated Materials and Theoretical Spectroscopy

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Hund metals have attracted attention in recent years due to their unconventional superconductivity, which supposedly originates from non-Fermi-liquid (NFL) properties of the normal state. When studying Hund metals using dynamical mean-field theory, one arrives at a self-consistent Hund impurity problem involving a multiorbital quantum impurity with nonzero Hund coupling interacting with a metallic bath. If its spin and orbital degrees of freedom are screened at different energy scales, T-sp < T-orb, the intermediate energy window is governed by a novel NFL fixed point, whose nature had not yet been clarified. We resolve this problem by providing an analytical solution of a paradigmatic example of a Hund impurity problem, involving two spin and three orbital degrees of freedom. To this end, we combine a state-ofthe-art implementation of the numerical renormalization group, capable of exploiting non-Abelian symmetries, with a generalization of Affleck and Ludwig's conformal field theory (CFT) approach for multichannel Kondo models. We characterize the NFL fixed point of Hund metals in detail for a Kondo model with an impurity forming an SU(2) x SU(3) spin-orbital multiplet, tuned such that the NFL energy window is very wide. The impurity's spin and orbital susceptibilities then exhibit striking power-law behavior, which we explain using CFT arguments. We find excellent agreement between CFT predictions and numerical renormalization group results. Our main physical conclusion is that the regime of spin-orbital separation, where orbital degrees of freedom have been screened but spin degrees of freedom have not, features anomalously strong local spin fluctuations: the impurity susceptibility increases as chi(imp)(sp) similar to omega(-gamma), with gamma > 1.

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