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Secondary aerosol formation in winter haze over the Beijing-Tianjin-Hebei Region, China

出版社

HIGHER EDUCATION PRESS
DOI: 10.1007/s11783-020-1326-x

关键词

Secondary aerosol formation; Regional haze; Photochemical reaction; Aqueous reaction; Chemical mechanism

资金

  1. National Natural Science Foundation of China [91844301, 91544214]
  2. National Research Program for Key Issues in Air Pollution Control [DQGG0103]
  3. National Key Research and Development Program of China [2016YFC0202000]

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This paper discusses the severe haze pollution in the Beijing-Tianjin-Hebei region during winter, the mitigation actions taken by the Chinese government since 2013, and the importance of secondary aerosol components during haze episodes. It highlights the need for research on the mechanisms of secondary aerosol formation to effectively control particle pollution in the region.
Severe haze pollution occurs frequently in the winter over the Beijing-Tianjin-Hebei (BTH) region (China), exerting profound impacts on air quality, visibility, and human health. The Chinese Government has taken strict mitigation actions since 2013 and has achieved a significant reduction in the annual mean PM2.5 concentration over this region. However, the level of secondary aerosols during heavy haze episodes showed little decrease during this period. During heavy haze episodes, the concentrations of secondary aerosol components, including sulfate, nitrate and secondary organics, in aerosol particles increase sharply, acting as the main contributors to aerosol pollution. To achieve effective control of particle pollution in the BTH region, the precise and complete secondary aerosol formation mechanisms have been investigated, and advances have been made about the mechanisms of gas phase reaction, nucleation and heterogeneous reactions in forming secondary aerosols. This paper reviews the research progress in aerosol chemistry during haze pollution episodes in the BTH region, lays out the challenges in haze formation studies, and provides implications and directions for future research. (c) Higher Education Press 2020

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