期刊
NATURE COMMUNICATIONS
卷 11, 期 1, 页码 -出版社
NATURE RESEARCH
DOI: 10.1038/s41467-020-19125-w
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资金
- MURI Center for Dynamic Magneto-optics
- Air Force Office of Scientific Research [FA9550-12-1-0119, FA9550-14-1-0040]
- DURIP grant [FA9550-15-1-0307]
- NSF [NSF1947070]
The subject of electromagnetism has often been called electrodynamics to emphasize the dominance of the electric field in dynamic light-matter interactions that take place under non-relativistic conditions. Here we show experimentally that the often neglected optical magnetic field can nevertheless play an important role in a class of optical nonlinearities driven by both the electric and magnetic components of light at modest (non-relativistic) intensities. We specifically report the observation of magneto-electric rectification, a previously unexplored nonlinearity at the molecular level which has important potential for energy conversion, ultrafast switching, nano-photonics, and nonlinear optics. Our experiments were carried out in nanocrystalline pentacene thin films possessing spatial inversion symmetry that prohibited second-order, all-electric nonlinearities but allowed magneto-electric rectification. The role of the optical magnetic field is generally not considered at nonrelativistic light intensities. Here the authors show magneto-electric rectification, an optical nonlinear effect due to electric and magnetic field coupling, in a thin film of the organic semiconductor pentacene at non-relativistic intensities.
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