期刊
SYNTHESIS-STUTTGART
卷 53, 期 1, 页码 51-64出版社
GEORG THIEME VERLAG KG
DOI: 10.1055/s-0040-1707234
关键词
copper catalysis; C-H bond functionalization; amination; nitrogen-fluorine bond; radical fluorination
资金
- Ministerio de Economia y Competitividad (MINECO) [CTQ2017-82893-C2-1-R]
- Universidad de Huelva [2014-2020 UHU-1254043]
This Short Review provides an update on copper-catalyzed C-H functionalization involving nitrogen-centered radicals from substrates containing N-F bonds. The processes discussed include intermolecular Csp(3)-H bond functionalization, remote Csp(3)-H bond functionalization via intramolecular hydrogen atom transfer (HAT), and Csp(2)-H bond functionalization, showing potential for future industrial applications.
This Short Review is aimed at giving an update in the area of copper-catalyzed C-H functionalization involving nitrogen-centered radicals generated from substrates containing N-F bonds. These processes include intermolecular Csp(3)-H bond functionalization, remote Csp(3)-H bond functionalization via intramolecular hydrogen atom transfer (HAT), and Csp(2)-H bond functionalization, which might be of potential use in industrial applications in the future.
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