期刊
OPTICAL MATERIALS
卷 107, 期 -, 页码 -出版社
ELSEVIER
DOI: 10.1016/j.optmat.2020.110029
关键词
Carbon dots; Microwave synthesis; Hematin detection; Inner filter effect
资金
- National Natural Science Foundation of China [41763020]
- Foundation of Jiangxi Educational Commission [GJJ180596]
Fluorescent carbon dots (CDs) are promising zero-dimensional carbon nanomaterials with semiconductor-like properties, which have attracted tremendous attention owing to their fascinating features such as excellent optical performance, chemical inertness, and low toxicology. In this investigation, Mg-doped CDs (Mg-CDs) with up- and down-conversion fluorescence (FL) were prepared within 2 min through a one-pot, facile and ultrafast microwave method. The obtained Mg-CDs showed excitation-independent blue emission and were potentially applied for the detection of hematin based on the strong inner filter effect (IFE). The FL intensity ratio (I-0/I) of the synthesized Mg-CDs were proportional to the concentration of hematin in the range of 0.1-75 mu M with the limit of detection of 25 nM for Mg-CDs-0.1 and 0.01-25 mu M with the limit of detection of 1 nM for Mg-CDs-0.5. Overall, this selective and sensitive assay using Mg-CDs obtained through the current microwave method was believed to demonstrate significant application prospects in complex matrices owing to its simplicity and specificity for hematin.
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