4.6 Article

Plasma synthesis of highly dispersed Pt nanoparticles on reduced graphene oxide-molybdenum disulfide nanosheets as efficient electrocatalysts for methanol oxidation reaction

期刊

MATERIALS LETTERS
卷 276, 期 -, 页码 -

出版社

ELSEVIER
DOI: 10.1016/j.matlet.2020.128258

关键词

Plasma; Graphene; Molybdenum disulfide (MoS2); Nanoparticles; Oxidation

资金

  1. National Natural Science Foundation of China [11635013, 11575253]
  2. Anhui Provincial Key Research and Development Plan [1704a0902017]
  3. PIFI Postdoc Fellowship [2020PE0031]

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Platinum/reduced graphene oxide-molybdenum disulfide composite (Pt/rGO-MoS2) is synthesized by employing H-2-plasma technique. The morphology, structure and component of Pt/rGO-MoS2 are investi-gated. Compared with Pt/rGO or Pt/MoS2, the as-prepared Pt/rGO-MoS2 catalyst exhibits large electro-chemical active area (104.3 m(2) g(-1)), high current density (737.8 mA mg(-1)) for methanol oxidation reaction (MOR) and long-term stability. These improvements are attributed to the rGO-MoS2 support that improves the dispersion of Pt NPs and offers sufficient electronic conductive channels. With these excel-lent electrochemical performances, this work may therefore offer a promising electrocatalyst for large-scale commercial application of fuel cells. (C) 2020 Elsevier B.V. All rights reserved.

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