期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 142, 期 42, 页码 17903-17907出版社
AMER CHEMICAL SOC
DOI: 10.1021/jacs.0c08058
关键词
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资金
- National Natural Science Foundation of China [21404062]
- Natural Science Foundation of Zhejiang Province [LY20B040003]
- Natural Science Foundation of Jiangsu Province [BK20171332]
Despite rapid progress in recent years, it has remained challenging to prepare well-defined metal-organic complex-based suprastructures. As a result, the physicochemical mechanisms leading to their geometrical complexity remain perplexing. Here, a porphyrin-based metallacage was used as a building block to construct octahedra via self-assembly, and the mechanism for the evolution of the metallacages into octahedra was disclosed by both experiments and theoretical simulations.
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