期刊
JOURNAL OF POWER SOURCES
卷 474, 期 -, 页码 -出版社
ELSEVIER
DOI: 10.1016/j.jpowsour.2020.228603
关键词
Perovskite fluoride; Carbon nanotubes; Specific capacity; Supercapacitors
资金
- National Natural Science Foundations of China [21673263, 21805291]
- Western Young Scholars Foundations of Chinese Academy of Sciences
- Youth Science Foundations of Gansu Province [18JR3RA389]
A series of KNiF3@carbon nanotubes (CNTs) are synthesized via a facile solvothermal method and applied as supercapacitor electrodes. The addition of carbon nanotubes can significantly overcome the rate capability defect of bare KNiF3 and improve the specific capacity to a certain extent, which mainly owing to the increase of conductivity and electron/ion transports capacity. In addition, the cross-linked structure of carbon nanotubes and the evenly anchoring of KNiF3 nanoparticles can increase the stability of the composites. As a result, the optimal candidate KNiF3@CNTs-8 (the content of carbon nanotubes is 8 mg and the mass fraction is 1.0%) shows highest specific capacity (821.4 C g(-1) at 1 A g(-1)) and capacity retention (83.6% at 16 A g(-1)). The asymmetric supercapacitor AC//KNiF3@CNTs-8 delivers extremely high energy density of 63.7 Wh kg(-1). More importantly, the ASC device shows ultra-long cycling stability, with 95.9% capacity retention after 5000 cycles. These results prove that KNiF3@CNTs can be a promising material for supercapacitor.
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