期刊
JOURNAL OF NANOPARTICLE RESEARCH
卷 22, 期 9, 页码 -出版社
SPRINGER
DOI: 10.1007/s11051-020-04961-0
关键词
Polyoxometalate; Ionic liquid; Heterogeneous oxidative desulfurization; Hydroxyapatite; Nanostructured catalysts; Environmental effects
资金
- Hainan Provincial Department of Science and Technology [ZDYF2018013]
- National Natural Science Foundation of China [21766007, 21776116]
- Commonwealth Scholarship Commission [201808460066, 201808460067]
With the continual air pollution and environmental issues caused by the combustions of sulfur-containing fuels, the desulfurization in transport fuels becomes a crucial topic worldwide. In this study, a kind of phosphomolybdic ionic liquid-supported hydroxyapatite was successfully designed and employed as a catalyst for heterogeneous oxidative desulfurization in fuel. The prepared catalysts were characterized via Fourier-transform infrared spectroscopy (FT-IR), X-ray diffraction (XRD), and Brunauer-Emmett-Teller (BET), which confirmed that phosphomolybdic ionic liquid was successfully immobilized on hydroxyapatite. With the prepared sample n-[Pmim]PMo/HAP, the sulfur removal could reach 97.2% under mild conditions. Furthermore, the supported catalyst has excellent recyclability and utilization foreground.
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