期刊
JOURNAL OF MATERIALS SCIENCE
卷 56, 期 2, 页码 1481-1491出版社
SPRINGER
DOI: 10.1007/s10853-020-05343-6
关键词
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资金
- National Natural Science Foundation of China [61367004]
- Guangxi Natural Science Foundation [2018GXNSFAA138127]
- State Key Laboratory of Luminescence and Applications [SKLA-2019-06]
Exciton localization phenomena were investigated in InGaN/GaN multiple-quantum-well structures with discrete quantum dots, showing enhanced localization within the dots and the impact of free carrier recombination. Non-exponential decay in TRPL measurements was explained using a model incorporating localized exciton, non-radiative, and free carrier recombination rates, proposing a new method to calculate internal quantum efficiency.
Exciton localization phenomena are considered here to comprehend the high internal quantum efficiency in InGaN/GaN multiple-quantum-well structures having discrete quantum dots (QDs) prepared by metal-organic-chemical-vapor deposition method onc-sapphire substrates. Spectroscopic results from the variable-temperature steady-state-photoluminescence and time-resolved photoluminescence (TRPL) are investigated. While the exciton localization is enhanced by strong localized states within the InGaN/GaN QDs-the impact of free carrier recombination cannot be ignored. The observed non-exponential decay in TRPL measurements is explained using a model by meticulously including localized exciton, non-radiative and free carrier recombination rates. A new method is proposed to calculate the internal quantum efficiency, which is supplementary to the traditional approach based on temperature-dependent photoluminescence measurement.
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