期刊
JOURNAL OF HAZARDOUS MATERIALS
卷 407, 期 -, 页码 -出版社
ELSEVIER
DOI: 10.1016/j.jhazmat.2020.124346
关键词
Disinfection byproduct; N-nitrosamines; HRMS; Water reuse; Chloramine
资金
- Spanish Ministry of Science, Innovation and Universities
- AEI-MICIU
- European Fund for Regional Development under the National Program for Research Aimed at the Challenges of Society, through the project NDMA_Predict [CTM2017-85335-R]
- Generalitat de Catalunya through Consolidated Research Groups [ICRA_ENV 2017 SGR 1124, ICRA_Tech 2017 SGR 1318]
- CERCA program
- Ramon y Cajal fellowship from the AEI-MICIU [RyC-2015-17108]
- European Union's Horizon 2020 research and innovation program under the Marie Sklodowska-Curie grant [839709]
A full-scale trial was conducted in summer 2019 to investigate the effects of discharging tertiary treated wastewater into the Llobregat River on drinking water quality. The study found that while the river contained low concentrations of NDMA, the NDMA precursors were already present at high levels. The concentration of NDMA in the drinking water was consistently low, but the formation potential varied.
In summer 2019, a full-scale trial was carried out to investigate the effects in drinking water quality when tertiary treated wastewater was discharged into the Llobregat River upstream of the intake of one of the major drinking water treatment plants of Barcelona and its metropolitan area. Two scenarios were investigated, i.e. discharging the reclaimed water with and without chemical disinfection with chlorine. This study investigates the concentration of N-nitrosodimethylamine (NDMA) as the specific disinfection conditions employed in this trial may favor its formation. To this aim, both NDMA and NDMA formation potential, were measured. The river contained NDMA at very low concentrations, but the concentration of NDMA precursors was already high. The NDMA concentration was reduced from discharge to the river to drinking water intake probably due to a combined effect of dilution and photolysis. The formation potential was also reduced probably due to dilution and biodegradation. The concentration of NDMA in the drinking water was always low (<7.3 ng/L), although the formation potential was above 10 ng/L in one sample. Dissolved organic matter characterization by high resolution mass spectrometry revealed differences between the nature of the organic matter in the river before and after reclaimed water discharge.
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