期刊
JOURNAL OF COLLOID AND INTERFACE SCIENCE
卷 577, 期 -, 页码 279-289出版社
ACADEMIC PRESS INC ELSEVIER SCIENCE
DOI: 10.1016/j.jcis.2020.05.077
关键词
Surface defect states; Fermi level; Heterojunctions; Self-powered photodetectors
资金
- National Natural Science Foundation of China [51871167, 51971158, 51702235]
- Natural Science Foundation of Tianjin [18JCYBJC86200]
- Scientific Developing Foundation of Tianjin Education Commission [2017ZD14]
Self-powered ultraviolet (UV) photodetectors (PDs) based on ZnO heterojunctions have attracted more attention due to the simple preparation and excellent photoresponse performance without any power supply. The self-powered UV PDs based on NiO nanoflakes/ZnO nanorod arrays (NRs) heterojunctions were fabricated by a low-cost, simple chemical bath deposition (CBD) method. The crystal quality, optical and electronic properties of ZnO NRs is modified by Al3+ ions additions in the precursor solution. The heterojunction devices with ZnO NRs grown in 0.5% Al3+ ions additions precursor solution exhibit a narrow UV spectral selectivity, high photoresponsivity R (85.12 mA/W) and detectivity D* (1.74 x 10(12) cm.Hz(1/2)/W) and a fast response speed (similar to 2 ms) under 378 nm UV light for low intensity irradiance (0.2 mW/cm(2)) at zero bias. The large built-in electric field of the NiO/ZnO heterojunction with the increased Fermi level of ZnO NRs provide a strong driving force to separate and transfer the photo-generated carriers, decrease the recombination of the carriers and then improve the photoresponse performance of heterojunction devices without external bias. (C) 2020 Elsevier Inc. All rights reserved.
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