期刊
ENVIRONMENTAL RESEARCH
卷 189, 期 -, 页码 -出版社
ACADEMIC PRESS INC ELSEVIER SCIENCE
DOI: 10.1016/j.envres.2020.109950
关键词
Antimony; Anaerobic and aerobic; Microbial extracellular polymeric; substances@Fe3O4; Nano zero-valent iron; Reduction efficiency
资金
- National Natural Science Foundation of China [51878212, 51578179]
- Open Project of State Key Laboratory of Urban Water Resource and Environment, Harbin Institute of Technology [ES201807]
The extracellular polymeric substances coating magnetic powders-supported nano zero-valent iron (nZVI@EPS@Fe3O4) was synthesized, using reduction and adsorption to treat Sb(V) wastewater. The adsorption performance and mechanism were investigated under aerobic and anaerobic conditions. The adsorption capacity of nZVI@EPS@Fe3O4 (79.56 mg/g at pH = 5) was improved compared to that of the original materials (60.74 mg/g). The spectral analysis shows that both nZVI and EPS@Fe3O4 in nZVI@EPS@Fe3O4 played an important role in reducing Sb(V) to Sb(III) and adsorbing Sb. The reducibility and adsorption capacity of nZVI@EPS@Fe3O4 towards Sb(V) remained strong under aerobic condition (62% Sb(III), 79.56 mg/g), although they were slightly weaker than those under anaerobic condition (74% Sb(III), 91.78 mg/g). nZVI@EPS@Fe3O4 showed good performance in regeneration experiments. nZVI@EPS@Fe3O4 is promising as a cost-effective and highly efficient material for Sb(V)-contaminated water. This study is meaningful in understanding the redox behaviour of nZVI composites in aerobic and anaerobic conditions.
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