期刊
ENERGY & FUELS
卷 34, 期 10, 页码 11942-11961出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.energyfuels.0c02647
关键词
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资金
- National Key Research and Development Program of China [2016YFB0100203]
- National Natural Science Foundation of China [21922508, 21673116, 21633003, U1801251]
- Natural Science Foundation of Jiangsu Province of China [BK20190009]
- Fundamental Research Funds for the Central Universities [14380176]
The lithium-sulfur (Li-S) battery has long been a research hotspot due to its high theoretical specific capacity, low cost, and nontoxicity. However, there are still some challenges impeding the Li-S battery from practical application, such as the shuttle effect of lithium-polysulfides (LiPSs), the growth of lithium dendritic, and the potential leakage risk of liquid electrolytes. Substitution of liquid electrolytes with solid-state electrolytes (SSEs) is an effective strategy to relieve or even solve these problems. This review focuses on the most crucial issues of the solid-state Li-S battery (SSLSB) and exhibits the recent progress in these fields. SSEs applicable in the Li-S battery including inorganic glassy ceramics and ceramics, organic polymers, and inorganic-organic hybrid electrolytes are reviewed. Then, the establishment of Li-ion pathways inside the cathode is discussed in detail. We also probe into the unique polysulfide chemistry of the Li-S battery and expound our opinions. Finally, conclusions and perspectives are outlined for the further development of SSLSBs.
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