期刊
ENERGIES
卷 13, 期 17, 页码 -出版社
MDPI
DOI: 10.3390/en13174511
关键词
CCS; carbon storage; injectivity; hydrate formation; flow remediation; CO2; CH4
资金
- Research Council of Norway (CLIMIT project) [255490]
- Equinor
Successful geological sequestration of carbon depends strongly on reservoir seal integrity and storage capacity, including CO(2)injection efficiency. Formation of solid hydrates in the near-wellbore area during CO(2)injection can cause permeability impairment and, eventually, injectivity loss. In this study, flow remediation in hydrate-plugged sandstone was assessed as function of hydrate morphology and saturation. CO(2)and CH(4)hydrates formed consistently at elevated pressures and low temperatures, reflecting gas-invaded zones containing residual brine near the injection well. Flow remediation by methanol injection benefited from miscibility with water; the methanol solution contacted and dissociated CO(2)hydrates via liquid water channels. Injection of N(2)gas did not result in flow remediation of non-porous CO(2)and CH(4)hydrates, likely due to insufficient gas permeability. In contrast, N(2)as a thermodynamic inhibitor dissociated porous CH(4)hydrates at lower hydrate saturations (<0.48 frac.). Core-scale thermal stimulation proved to be the most efficient remediation method for near-zero permeability conditions. However, once thermal stimulation ended and pure CO(2)injection recommenced at hydrate-forming conditions, secondary hydrate formation occurred aggressively due to the memory effect. Field-specific remediation methods must be included in the well design to avoid key operational challenges during carbon injection and storage.
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