期刊
BIORESOURCE TECHNOLOGY
卷 311, 期 -, 页码 -出版社
ELSEVIER SCI LTD
DOI: 10.1016/j.biortech.2020.123520
关键词
Tea Residue; Hydrogel; Adsorption Mechanism; Fixed-Bed Column
资金
- National Key Research and Development Project [2017YFC1600702]
A novel macroporous (similar to 150 mu m) double network hydrogel (TR/PAA) was prepared from tea residue and acrylic acid, and its performance was systematically evaluated. The static adsorption experiments showed that gel exhibited high selectivity and adsorption capacity, ultrafast kinetics (similar to 10 min) for Cr(III), Pb(II) and Fe(III). The adsorption behavior showed heterogeneous and chemisorption process adsorption capacities of 206.19, 253.16, and 94.88 mg g(-1) for Cr(III), Pb(II) and Fe(III), respectively. In pluralistic systems, TR/PAA showed the adsorption order of Fe(III) > Cr(III) > Pb(II). Mechanism studies confirm that nitrogen and oxygen-containing functional groups play a major role in the adsorption process. In the fixed-bed column experiments, the treatment volume of simulated wastewater reached 1400 bed volumes (BV) (21.6 L), producing only 7 BV (323 mL) eluent. This work provides a new avenue for the combination of TR/PAA reuse and heavy metal removal, which is expected to be applied in actual wastewater treatment.
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