期刊
ADVANCED FUNCTIONAL MATERIALS
卷 30, 期 49, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adfm.202003055
关键词
anion sorbents; lithium batteries; metal-organic frameworks; particulate additives
类别
资金
- UCLA-HK Center for Graphene Technology and Energy Storage
The performance of lithium batteries is heavily governed by the transport of ions within the electrolytes. Commercial liquid electrolytes, however, generally exhibit a low lithium-ion transference number, causing concentration polarization, side reactions, and deteriorated battery performance. Herein, a novel class of electrolyte additives based on particles of metal-organic framework is proposed to immobilize the anions while allowing efficient transport of lithium ions in the electrolytes. The use of such additives effectively increases the lithium-ion transference number, enhances the rate capability, and prolongs the cycling life, which provides a facile yet effective strategy toward lithium batteries with dramatically improved performances.
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