期刊
FRONTIERS IN CHEMISTRY
卷 8, 期 -, 页码 -出版社
FRONTIERS MEDIA SA
DOI: 10.3389/fchem.2020.00437
关键词
two-dimensional; metal-free; electrocatalyst; N(2)fixation; Faradaic efficiency
资金
- National Natural Science Foundation of China [21535004, 91753111, 21927811, 21390411, 21301110]
- Natural Science Foundation of Shandong Province of China [ZR2013BQ011]
The ever-growing requirement of ammonia for industry and energy supply motivates people to find clean and cost-effective alternatives to overcome the shortcomings of the century-old Haber-Bosch process. Electrocatalytic N(2)reduction (NRR) is considered a prospective way for ammonia production at ambient conditions. Recently, two-dimensional (2D) metal-free materials are emerging as highly efficient and robust electrocatalysts for NRR owing to their advanced features: highly exposed surface, abundant active sites, tunable electronic states, and long-term stability compared to metal-based and bulk catalysts. In this minireview, we briefly summarize the latest edge reports on 2D metal-free materials catalyzed NRR. Also, we discuss the challenges and perspectives on the design and synthesis of novel 2D metal-free catalysts.
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