Evolution of flame-kernel in laser-induced spark ignited mixtures: A parametric study

The present work focuses on the early stages of flame-kernel development in laser-induced spark ignited mixtures issuing out of a Bunsen burner. The time-scale of 3 mu s to 1 ms associated with the flame-kernel evolution stage of an ignition event is targeted in this work. A CH4/air mixture (equivalence ratio phi = 0.6) is studied as a base case, and compared with CH4/CO2/air (mole fractions = 0.059/0.02910.912, respectively) and CH4/H-2/air (mole fractions = 0.053/0.016/0.931, respectively) mixtures for nearly the same adiabatic flame temperature of 1649 K. The spatio-temporal flame-kernel evolution is imaged using planar laser induced fluorescence of the OH radical (OH-PLIF), simultaneously with H-alpha emission from the plasma. The H-alpha emission suggests that the plasma time-scale is well below 1 mu s. The PLIF images indicate all the stages of kernel development from the elongated kernel to the toroidal formations and the subsequent appearance of a front-lobe. The different time-scales associated with these stages are identified from the rate of change of the kernel perimeter. The plasma is followed by a supersonic kernel-perimeter growth. Larger flame-kernel spread is found in the case of CH4/H-2 mixtures. A distinct shift in the trends of evolution of LIF intensity and kernel perimeter is observed as the fuel concentration is varied near the lean flammability limit in CH4/air (phi = 0.35-0.65) and H-2/air (phi = 0.05-0.31) mixtures. The flow velocity (Reynolds number, Re) effect in both laminar and turbulent flow regimes (Re = similar to 600-6000) indicates that the shape of the flame-kernel changes at higher velocities, but the size of the kernel does not change significantly for a given time from the moment of ignition. This could be due to a balance between two competing effects, namely, increase in the strain rate that causes local extinction and thus decreases the flame-kernel growth, and increase in the turbulence levels that facilitates increased flame-kernel surface area through wrinkling, which in turn increases the flame-kernel growth. (C) 2015 The Authors. Published by Elsevier Inc. on behalf of The Combustion Institute. This is an open access article under the CC BY license (http://creativecommons.org/licenses/by/4.0/).