期刊
ORGANIC LETTERS
卷 22, 期 17, 页码 6734-6738出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.0c02091
关键词
-
资金
- National Natural Science Foundation of China [21801154]
- Natural Science Foundation of Shandong Province [ZR 201709190401]
Herein reported is a nickel-catalyzed reductive aryl thiocarbonylation of alkene via thioester group transfer strategy by using simple and readily available thioesters. In contrast to traditional activation of weaker C(acyl)-S bond, the C(acyl)-C bond of thioester was selectively cleaved to enable this reaction under mild conditions. Furthermore, this approach features operational simplicity and broad substrate scope, providing a complementary and practical route for thioester synthesis without requiring toxic thiol or CO gas.
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