期刊
ORGANIC LETTERS
卷 22, 期 14, 页码 5675-5679出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.0c02069
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-
资金
- Ministry of Science and Technology of the Republic of China [104-2628-M-003-001-MY3, 107-2113-M-003-014-MY3]
Reported herein is a method for the efficient syntheses of optically active 1-alkyl homoallylic amines in yields up to 95%, 13.5:1 dr, and 98% ee under mild, aqueous reaction conditions, via the Rh-catalyzed asymmetric allylation of aliphatic aldimines. This method provides a streamlined synthetic platform for the preparation of indolizidine and piperidine alkaloids, thus demonstrating its usefulness.
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