期刊
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
卷 45, 期 46, 页码 24870-24882出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.ijhydene.2020.06.264
关键词
Two-stage adsorption process; CO2 capture; H-2 production; Silica gel; Zeolite 5A; Activated carbon
资金
- Renewable Energy and Hydrogen Projects in National Key RD Plan of China [2019YFB1505000]
A two-stage vacuum/pressure swing adsorption (VSA/PSA) process has been investigated for CO2 capture and then H-2 production from steam methane reforming (SMR) gas mixture. The target is to produce ultra-pure hydrogen and high-purity CO2. Many fundamental research studies have been carried out to validate the accuracy of numerical calculation, such as isotherm measurement, fitting and process modelling. The results indicate that the first stage process could produce 95.31% CO2 with the recovery of 90.93% and the second stage could produce 99.9952% H-2 with an overall recovery of 71.16%. Variable analysis, optimal conditions and comparison with other processes are discussed in detail. (C) 2020 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
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