期刊
CLEAN TECHNOLOGIES AND ENVIRONMENTAL POLICY
卷 18, 期 6, 页码 1889-1903出版社
SPRINGER
DOI: 10.1007/s10098-016-1117-z
关键词
Sonophotocatalysis; Acid yellow 23; Fe/Zinc oxide composite; Colour removal; Real textile effluent; COD reduction
资金
- Ministry of Environment and Forest (MoEF), Government of India
Nanocatalysts such as ZnO, Fe and Fe/ZnO composite were synthesized for better treatment of dye than the conventional treatment methods. The catalysts were characterized using SEM, EDAX, BET surface area, XRD and DRS. The degradation of acid yellow 23 dye in aqueous solution has been investigated using sonolysis, photolysis and sonophotocatalysis. The effect of different conventional operating parameters such as initial solution pH, gas purging (Argon, Oxygen, Air and Nitrogen) and H2O2 addition, under sonolysis (13 and 25 mm probe tip diameter) and photolysis (UV light), showed a maximum of 41 % colour removal for 0.0187 mmol/L dye solution under photolysis with 88.2 mmol/L H2O2 addition. Among the catalysts used, 98 % dye colour removal was obtained with 0.2 g/L Fe/ZnO composite under 60 min of sonophotolysis that had been benefitted by the synergistic effects. The HPLC spectrum of the untreated dye and treated dye supports the claim of eradication of the parent dye compound. Sonophotocatalytic treatment of real textile effluent in the presence of 6 g/L Fe/ZnO composite and 264.6 mmol/L H2O2 reduced the COD level from 792 to 174.4 mg/L in 240 min to meet the allowable effluent discharge standard into running water streams. The studied treatment methods were found to be effective for the degradation of acid yellow 23 dye and subsequently in real textile effluent too.
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