期刊
ELECTROCHEMISTRY COMMUNICATIONS
卷 115, 期 -, 页码 -出版社
ELSEVIER SCIENCE INC
DOI: 10.1016/j.elecom.2020.106734
关键词
Electrosynthesis; Proton-exchange membrane (PEM) reactor; Electrocatalytic asymmetric hydrogenation; alpha,beta-Unsaturated acids; Cinchona-modified palladium catalysts
资金
- JST CREST Grant, CREST, Japan [JP65R1204400]
- [2707]
We have developed an electrocatalytic asymmetric hydrogenation reaction using a proton-exchange membrane (PEM) reactor that employs a polymer electrolyte fuel cell and industrial electrolysis technologies. Reasonable enantioselectivities and excellent current efficiencies were obtained in the asymmetric hydrogenation of alpha-phenylcinnamic acid under mild conditions without adding a supporting electrolyte. The current density was crucial to achieving the improved results observed.
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