期刊
CHINESE JOURNAL OF ORGANIC CHEMISTRY
卷 36, 期 5, 页码 889-912出版社
SCIENCE PRESS
DOI: 10.6023/cjoc201511017
关键词
diazo compounds; transition-metal-catalysis; C-H activation; alkyaltion
资金
- National Natural Science Foundation of China [21302064]
- Scientific Research Project of Hubei Provincial Department of Education [B2015231]
Diazo compounds had been widely employed as a class of environment friendly and highly efficient coupling reagents in transition-metal-catalyzed C-H bonds insertion reactions. Recently, C-H alkylation of various arenes and heteroarenes has been achieved enormous successes using diazo compounds as the alkylation reagents under a new catalytic model. The recent progress in diazo compounds mediated transition-metal-catalyzed C-H alkylation and tandem C-H alkylation/cyclization is reviewed, including reaction mechanism and synthetic applications. Furthermore, the prospects of this reaction are also discussed.
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