期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 59, 期 44, 页码 19380-19389出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.202005776
关键词
ADOR approach; germanosilicates; hydrolysis; zeolites
资金
- Charles University Centre of Advanced Materials (CUCAM-OP VVV Excellent Research Teams) [CZ.02.1.01/0.0/0.0/15_003/0000417]
- Primus Research Program of the Charles University [PRIMUS/17/SCI/22]
- Czech Science Foundation [20-12099S, 19-27551X, 19-21534S]
- National Natural Science Foundation of China [U1967215, 21835002, 21621001]
- 111 Project of China [B17020]
Zeolites are one of the most important heterogeneous catalysts, with a high number of large-scale industrial applications. While the synthesis of new zeolites remain rather limited, introduction of germanium has substantially increased our ability to not only direct the synthesis of zeolites but also to convert them into new materials post-synthetically. The smaller Ge-O-Ge angles (vs. Si-O-Si) and lability of the Ge-O bonds in aqueous solutions account for this behaviour. This Minireview discusses critical aspects of germanosilicate synthesis and their post-synthesis transformations to porous materials.
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