期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 60, 期 20, 页码 11036-11047出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.202006472
关键词
artificial interphases; batteries; electrolytes; magnesium-ion batteries
资金
- University of Colorado Boulder College of Engineering & Applied Science and Engineering
- Paul M. Rady Department of Mechanical Engineering
The development of rechargeable magnesium batteries has been hindered by the incompatibility between the magnesium-metal anode and conventional carbonate electrolytes. Research is focused on finding thermodynamically stable electrolytes while developing methods for artificial solid-electrolyte interphase.
The first prototype of a rechargeable magnesium (Mg) battery demonstrated two decades ago sparked tremendous interest in the electrochemical community due to their potential low cost, high volumetric energy density. However, the development of rechargeable Mg batteries has been hampered by the incompatibility between the Mg-metal anode and conventional carbonate electrolytes. Research has focused on electrolytes that are thermodynamically stable against reduction at the expense of low oxidation potential at the cathode side. Alternatively, the use of an artificial solid-electrolyte interphase (SEI) via surface coating presents promising results to address the Mg/electrolyte incompatibility and significantly broaden the selection of electrolytes. This minireview discusses the limitations of electrolyte development and strategies for the design of artificial interphases in magnesium-ion batteries. Future perspectives in the development of artificial interphases for rechargeable magnesium batteries are also discussed.
作者
我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。
推荐
暂无数据