期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 59, 期 36, 页码 15298-15312出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.202007672
关键词
activities; electrocatalysis; nanoelectrochemistry; selectivities; stabilities
资金
- Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) [EXC 2033-390677874-RESOLV]
- collaborative research centre/transregio Heterogeneous Oxidation Catalysis in the Liquid Phase (TRR 247) [388390466]
- FOR 2982 within the research unit UNODE-unusual anode reactions [433304666]
- European Research Council (ERC) under the European Union [833408]
- Projekt DEAL
- European Research Council (ERC) [833408] Funding Source: European Research Council (ERC)
The use of renewable energy by means of electrochemical techniques by converting H2O, CO(2)and N(2)into chemical energy sources and raw materials, is the basis for securing a future sustainable green energy supply. Some weaknesses and inconsistencies in the practice of determining the electrocatalytic performance, which prevents a rational bottom-up catalyst design, are discussed. Large discrepancies in material properties as well as in electrocatalytic activity and stability become obvious when materials are tested under the conditions of their intended use as opposed to the usual laboratory conditions. They advocate for uniform activity/stability correlations under application-relevant conditions, and the need for a clear representation of electrocatalytic performance by contextualization in terms of functional investigation or progress towards application is emphasized.
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