期刊
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
卷 59, 期 37, 页码 15963-15967出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.202006530
关键词
chromophores; dimers; energy transfer; noncovalent interactions; supramolecular chemistry
资金
- Leverhulme Trust [RP2013-SL-008]
- ERC-2016 Consolidator Grant (CAM-RIG) [726470]
- Marie Sklodowska-Curie Fellowship (H2020-MSCA-IF-2018) [845640]
- EPSRC Programme Grant (NOtCH) [EP/L027151/1]
- European Research Council (ERC) [726470] Funding Source: European Research Council (ERC)
- EPSRC [EP/L027151/1] Funding Source: UKRI
- Marie Curie Actions (MSCA) [845640] Funding Source: Marie Curie Actions (MSCA)
The challenge of quantitatively forming self-assembled heterodimers without other equilibrium by-products is overcome through self-sorting favored by the introduction of designed shape-complementary moieties. Such a supramolecular strategy based on cucurbit[8]uril-directed dimerization is further applied to generate hetero-chromophore dimers quantitatively, leading to efficient energy transfer (>85 %) upon photoexcitation.
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