期刊
ADVANCED FUNCTIONAL MATERIALS
卷 30, 期 35, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adfm.202003430
关键词
anti-freezing; cellulose nanofibrils; ionic conductor; multi-functional sensors; strong and tough
类别
资金
- Canada Research Chairs program [231928]
- Natural Sciences and Engineering Research Council of Canada (NSERC) [RGPIN-2018-06818]
- Canada Foundation for Innovation-John R. Evans Leaders Fund (CFI-JELF) [37517]
- Four-Year Doctoral Fellowship (4YF) program at UBC
To date, ionic conducting hydrogel attracts tremendous attention as an alternative to the conventional rigid metallic conductors in fabricating flexible devices, owing to their intrinsic characteristics. However, simultaneous realization of high stiffness, toughness, ionic conductivity, and freezing tolerance through a simple approach is still a challenge. Here, a novel highly stretchable (up to 660%), strong (up to 2.1 MPa), tough (5.25 MJ m(-3)), and transparent (up to 90%) ionic conductive (3.2 S m(-1)) organohydrogel is facilely fabricated, through sol-gel transition of polyvinyl alcohol and cellulose nanofibrils (CNFs) in dimethyl sulfoxide-water solvent system. The ionic conductive organohydrogel presents superior freezing tolerance, remaining flexible and conductive (1.1 S m(-1)) even at -70 degrees C, as compared to the other reported anti-freezing ionic conductive (organo)hydrogel. Notably, this material design demonstrates synergistic effect of CNFs in boosting both mechanical properties and ionic conductivity, tackling a long-standing dilemma among strength, toughness, and ionic conductivity for the ionic conducting hydrogel. In addition, the organohydrogel displays high sensitivity toward both tensile and compressive deformation and based on which multi-functional sensors are assembled to detect human body movement with high sensitivity, stability, and durability. This novel organohydrogel is envisioned to function as a versatile platform for multi-functional sensors in the future.
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