期刊
CHEMISTRY OF MATERIALS
卷 28, 期 6, 页码 1920-1926出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.chemmater.6b00267
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资金
- STANDUP for Energy, the Swedish Research Council (VR)
- Swedish Foundation for Strategic Research
Dilithium benzenedipropiolate was prepared and investigated as a potential negative electrode material for secondary lithium-ion batteries. In addition to the expected reduction of its carbonyls, this material can reduce and reversibly oxidize its unsaturated carbon carbon bonds leading to a Li/C ratio of 1/1 and a specific capacity as high as 1363 mAh g(-1): the highest ever reported for a lithium carboxylate. Density functional theory calculations suggest that the lithiation is preferential on the propiolate carbons.
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